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List of Symbols and Abbreviations XIII
Introduction: Historical Remarks 1
Basic Concepts 7
Charge Transfer 7
Molecular Orbitals and Transfer Integrals 8
Structural Aspects 13
Molecular Building Blocks 13
Crystal Structures 16
Quasi-One-Dimensional Compounds 16
Quasi-Two-Dimensional Compounds 19
Three-dimensional Compounds 25
Anion Ordering and Glassy Phenomena 29
Normal-State Properties 37
Tight-Binding Model 37
Fermi Surfaces and Low Dimensionality 42
Electronic Properties 45
Transport and Optical Properties 45
Thermal and Magnetic Properties 63
Instabilities Involving Spin- and Charge-Degrees of Freedom 75
Charge- and Spin-Density-Waves 75
Spin-Peierls State 81
Charge-Ordering Phenomena 83
Many-Body Effects 87
Phase Diagrams 91
Magnetic-Field Effects 99
Electron Motion in Magnetic Fields 100
Semi-Classical Description in k-Space 100
Angular-Dependent Magnetoresistance Oscillations 101
Magneto-Optic Resonances 106
Magnetic Quantum Oscillations 109
Landau Levels and Lifshitz-Kosevich Theory 109
Magnetic Breakdown and Quantum Interference 117
Two-Dimensionality Effect 120
Superconducting Vortex States 123
Magnetic Exchange-Interaction 126
High-Magnetic Field States 128
Field-Induced Cascade Transitions to SDWs and Anomalous High-Field States 128
Field-Induced Destruction of CDW and Anomalous High-Field States 133
Approaching the Quantum Limit 138
Superconductivity 141
Occurrence of Superconductivity in Molecular Metals 141
Ginzburg-Landau Theory 143
The Superconducting Phase Transition 147
Anisotropy and Superconducting Fluctuations 148
Pressure Dependence of T[subscript c] 153
Disorder 157
Superconducting Parameters 164
(TMTSF)[subscript 2]X 165
(BEDT-TTF)[subscript 2]X and (BEDT-TSF)[subscript 2]X 166
The Superconducting Mixed State 170
Overview 170
Basic Concepts of Vortex Matter in Quasi-Two-Dimensional Systems 172
Experimental Findings for [kappa]-(BEDT-TTF)[subscript 2]X 175
Superconducting Order-Parameter 188
On the Pairing Mechanism 210
Phenomena of Interacting [pi]- and d-Electrons 219
(DCNQI)[subscript 2]Cu 219
Crystal Structure and Electrical Conductivity 219
Reentrant Metal-Insulator Transition 221
(BEDT-TSF)[subscript 2]FeX[subscript 4] (X=Cl,Br) 224
Crystal Structures and Transfer Integrals 225
Conductivity and Magnetism 227
Magnetic Interactions and Mean-Field Theories 229
Anomalous Metallic States 232
Antiferromagnetic Insulating States 236
Magnetic Field-Induced Transitions 241
Epilogue 247
References 249
Index 291
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