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Electronic Properties of Novel Materialsascience and Technology of Molecular Nanostructures ... Book

Electronic Properties of Novel Materialsascience and Technology of Molecular Nanostructures ...
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  • Electronic Properties of Novel Materialsascience and Technology of Molecular Nanostructures ...
  • Written by author Hans Kuzmany, Siegmar Roth, Jorg
  • Published by American Institute of Physics, 1999/10/01
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Preface xiii
Table of Previous Kirchberg Winterschools xiv
Organizer, Patronage, Supporters, and Sponsors xv
I. Fullerene Materials
The Jahn-Teller Distortion of [characters not reproducible] as Determined by ESR 3
Origin of Intrinsic Luminescence from C[subscript 60] Single Crystals 7
Polymeric Fullerenes: From C[subscript 60] to C[subscript 70] 12
In situ ATR-FTIR Spectroelectrochemical Comparison of Pristine and Polymerized C[subscript 60] Films 16
Structure of Phototransformed C[subscript 60] Revisited 20
Atomic Force Microscopy Analysis of Nucleation and Diffusion of C[subscript 60] on Hot Substrates 24
NMR Study of C[subscript 60].C[subscript 7]H[subscript 8] by Cross Polarization and Polarization Inversion of Rare-Spin Magnetization 28
Is the Ground State of A[subscript 1]C[subscript 60] (A=Rb, Cs) Antiferromagnetic? 32
Comparative Study of Ferromagnetic and Non-Ferromagnetic Modifications of TDAE-C[subscript 60] 37
Spin-Singlets in Metallic Cubic Quenched CsC[subscript 60] 42
Distinct Polymer Chain Orientations in KC[subscript 60] and RbC[subscript 60] 47
Low Symmetry Structures in the Li-Rb-C[subscript 60] Phase Field 52
Conduction Electron Spin Resonance in the Superconducting State of K[subscript 3]C[subscript 60] 56
Orientational Ordering of Alkali Ammonia Clusters in Ammoniated Alkali Fullerides (NH[subscript 3])K[subscript 3]C[subscript 60] and (ND[subscript 3])K[subscript 3]C[subscript 60] 60
Electronic Properties of the Na[subscript 2]AC[subscript 60] Family (A=K, Rb, Cs) 64
Structure and Physical Properties of Cs[subscript 3]C[subscript 60] under Ambient and High Pressures 69
Structural Studies of Superconducting Li[subscript 3]CsC[subscript 60] 73
Structure of Ca[subscript 4](NH[subscript 3])C[subscript 60] 78
II. Endohedral Fullerenes
Atoms in Molecular Cages 85
IR and Raman Analysis of Diatomic Encapsulates in Fullerene Cages 90
Endohedral Fullerenes with Lower Carbon Cage Sizes 95
Atoms in Fullerene Traps as Probes for Local Fields 101
Cerium Metallofullernes 106
The Electronic Properties of Charged N@C[subscript 60] 111
Structural and Magnetic Studies of the Endohedral Metallofullerene Ce@C[subscript 82] 115
Dynamic Motion of Ce@C[subscript 80]--Comparison Study with Ce@C[subscript 82] 120
Structural Phase Transitions of Endohedral Metallofullerene La@C[subscript 82] Studied by Single Crystal X-ray Diffraction
Endohedral Rare Earth Fullerenes--Electronic and Dynamic Properties 128
The Electronic Structure of Mono- and Dimetallofullerenes by Photoemission Spectroscopy 132
A Raman Study of Empty C[subscript 84] Isomers D[subscript 2] and D[subscript 2d] and Three Isomers of Sc[subscript 2]@C[subscript 84] 136
A Vibrational Spectroscopic Structure Analysis of Eu@C[subscript 74] 140
Light-Induced Release of Nitrogen from Fullerene Cages 144
Atomic Hydrogen in the Si[subscript 8]O[subscript 12] Cage 148
III. New Nanostructured Materials
Oligomer-Fullerene Dyads and Traids as Model Compounds for Bulk-Heterojunction TV Cells 155
Photo-Induced Charge-Transfer Processes in Fullerene-Containing Dyad and Triad Molecules 161
C[subscript 59]N on Silicon Surfaces: Monomers, Dimers, and Multilayers 165
Homonclear Bonds in BN Clusters? 170
Synthesis and Characterisation of Organometallic Compounds of Fullerene Derivatives 175
Non-IPR Fullerences: C[subscript 36] and C[subscript 72] 179
Effect of Alkali Doping on the Structural Stability of Solid C[subscript 36] 183
Isolation and Characterisation of [84]Fullerene Isomers 187
New Three-Component Systems Based on C[subscript 60] 191
Cluster-Assembled Amorphous Carbon Nano-Foam Synthesized by High-Pulse-Rate Laser Ablation 196
Self-Formation of Nanostructures from hydrated Aggregates and Nanocrystals of (C[subscript 60])[subscript n] Molecules on the Liquid Crystal Layer 200
Chains of Carbon Nanoparticles from the Interaction of Fullerenes with Thin Metal Films 205
Electrochemical Preparation of Carbon Chains and Nanoparticles 209
Preparation of Carbyne-Like Films by Dehydrochlorination of Poly(Vinylidene Chloride) 213
X-Ray Emission Spectroscopy Study of C[subscript 2]F Intercalated with Benzene 217
Vanadium Pentoxide Nanowires 221
Production and Investigation of Vanadium Pentoxide (V[subscript 2]O[subscript 5]) Nanostructures Grown in IR Laser-Field 226
Perfect Nanospheres from Polymerized Lipofullerenes 231
IV. Preparation and Characterization of Carbon Nanotubes
A Continuous Wave CO[subscript 2] Laser Reactor for Nanotubes Synthesis
Synthesis, Purification, and Characterisation of Multi- and Single-Wall Nanotubes Produced by Catalytic Decomposition of Hydrocarbons 241
Production of Bundles of Single Walled Nanotubes by a Simple Laser Ablation Technique 245
Metal Mixtures Catalysed Carbon Nanotube Synthesis 249
Solar Synthesis of Single Wall Carbon Naontubes 254
Carbon Arc Plasma Doped with Fe and Co/Ni: Spectroscopy and Formation of Carbon Nanostructures 258
Large Arrays of Well-Aligned Carbon Naontubes 263
Sulfur: The Key for Filling Carbon Naotubes with Metals 268
Alkali-Metal Intercalation in Carbon Nanotubes 273
About the Composition of Single Wall Carbon Nanotube Bundles: An Analysis from Optical, Raman, and IR Experiments 278
Polymers of Single Wall Nanotubes: Geometry, Diffraction Pattern, and Electronic Spectrum Modelling 284
The Characterization of SWNT Containing Soot by Optical Spectroscopy 288
Evolution of Carbon Single-Walled Nanotubes Diameter as a Function of the Synthesis Parameters: A Raman Study 292
V. Porperties of Carbon Nanotubes
Neutron Scattering Studies of Carbon Nanotubes 299
Statistical Analysis of the Electronic Structure of Single Wall Carbon Nanotubes in Buckypaper 304
Characterization of Single Wall Carbon Nanotubes by Scanning Tunneling and Scanning Force Microscopy 308
STM Investigation of Single-Wall Carbon Nanotubes at Room Temperature 313
Scanning Tunneling Microscopy of Carbon Nantubes: Simulation and Interpretation 319
The Use of Computer Simulation to Investigate Tip Shape and Point Contact Effects During Scanning Tunneling Microscopy of Supported Nanostructures 323
Optical Absorption and Resonance Raman Scattering of Carbon Nanotubes 328
In situ Raman Investigations of Single-Wall Carbon Nanotubes Pressurized in Diamond Anvil Cell 333
Surface Enhanced Raman Spectroscopy of Single Wall Carbon Nanotubes 338
Disorder Effects on Density of States and Electronic Conductance in Carbon Nanotubes 342
Electronic Structure Studies of Carbon Nanostructures Using Electron Energy-Loss Spectroscopy in Transmission 346
The Effects of Dimensionality on the [pi]-Plasmon-Dispersion in Multi-Wall Carbon Nanotubes 351
Molecular Mechanics Study of Carbon Nanotubes 355
Knock-on Damage in Single Wall Carbon Nanotubes by Electron Irradiation 360
Sliding, Stretching, and Tapering: Recent Structural Results for Carbon Nanotubes 364
VI. Electronics of Molecular Nanostructures
Temperature Dependence of the Resistivity of Individual Multi-Walled Pure/Boron Doped Carbon Nanotubes at Elevated Temperatures 371
Temperature Dependent Resistivity of Large Ropes of Single-Walled Carbon Nanotubes 375
Manipulation of the Transport Properties of Single-Walled Nanotubes by Alkali Intercalation and Local Charge Transfer 379
Femtosecond Time-Resolved Photoemission as a Probe of Electronic Transport in Single Wall Carbon Nanotubes 384
One-Dimensional Transport in Bundles of Single-Walled Carbon Nanotubes 388
Electrical Transport in Carbon Nanotube Rings: Coherence and Localization 393
Quantentransport in Multi-Wall Carbon Nanotubes 399
Electron Interference Effect in Multi-Wall Carbon Nanotubes 403
Charge Transport in Carbon Nanotube Transistors 407
Luttinger Liquid Behavior in Single-Wall Nanotubes 411
Electric Resistivity and Magnetoresistance of Some Superhard and Ultrahard Fullerites in the Range 300-2K 416
Electron Transport Through a Gold-Bisthiolterthiophene-Gold Junction 421
VII. Applications
Capacitance Properties of Carbon Nanotubes 429
Electron Field Emission from Carbon 433
Field Emission from Carbon Nanotubes and Its Application to Electron Sources 439
Thin Film Cold Cathode from Nanostructured Carbon 444
Field Emission Properties of Carbon Nanowires from ab initio Calculations 448
Electrocatalytic Properties of the C[subscript 60], C[subscript 70], C[subscript 76], C[subscript 78], and C[subscript 84] Fullerene Anions 452
Carbon Nanotubes and Gas Adsorption 456
Electrochemical Storage of Hydrogen in Carbon Single Wall Nanotubes 462
Characterization of Multi-Walled Carbon Nanotubes-PMMA Composites 466
Functionalisation of Carbon Nanotubes for Composites 470
Chemical Functionalization of Carbon Nanotubes 474
Electronic Structures and Applications of Carbon Nanotubes 478
Combinatorial Chemistry Approach to Development of Molecular Plastic Solar Cells 483
Charge Transfer and Relaxation Dynamics of Excited Electronic States in Organic Photoreceptor Materials With and Without C[subscript 60] 487
Optical Limiting Materials Based on Fullerene Derivatives 492
SPM Investigation of Superhard Carbon Prepared from C[subscript 60] Fullerene 497
Raman Spectrum and Stability of (C[subscript 59]N)[subscript 2] 501
Author Index 507


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